Technical Name |
Fabrication of high-capacity and high-safety lithium half-cells and pouch cells was achieved through the integrated development of anode materials, protective interlayers, and electrolyte systems. |
Project Operator |
NTHU-ChE |
Project Host |
胡啟章 |
Summary |
The closed-pore structure can be tuned by carbonization temperature, enabling a reversible low-potential plateau that boosts lithium-ion battery capacity while maintaining cycling stability. Electrospinning PAN protective layers, optimized via voltage control, improve lithium-ion transport and plating uniformity. The high-entropy ionic liquid shows excellent compatibility with NMC811 and Si–C electrodes, significantly enhancing battery safety. The performance of these materials ca be evaluated in the small pouch cell. |
Scientific Breakthrough |
Through structural design of hard carbon precursors, a reversible lithium-ion storage capacity of 680 mAh/g was achieved. The electrospinning protective layer maintained lithium thickness near theoretical values after extended plating, enabling precise control of lithium metal deposition. Meanwhile, the high-entropy ionic liquid enhanced battery safety without sacrificing capacity or cycle life. The 1 Ah pouch-cell platform validates the practical applicability of these combined innovations. Dual prelithiated silicon oxide (SiOx) materials can achieve an initial coulombic efficiency exceeding 96% and a specific capacity of 1600 mAh g⁻¹, enabling the use of fully SiOx-based anodes for practical lithium-ion battery design and applications |
Industrial Applicability |
Li-ion batteries of the next generation, high-performance Na-ion batteries, Li-ion capacitors, and Na-ion capacitors for the battery back unit (BBU) in the AI servers. |